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arXiv · 0901.1313

The chemical history of molecules in circumstellar disks. I. Ices

R. Visser·E. F. van Dishoeck·S. D. Doty·C. P. Dullemond
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Abstract

(Abridged) Aims & Methods. A two-dimensional, semi-analytical model is presented that follows, for the first time, the chemical evolution from a collapsing molecular cloud (a pre-stellar core) to a protostar and circumstellar disk. The model computes infall trajectories from any point in the cloud and tracks the radial and vertical motion of material in the viscously evolving disk. It includes a full time-dependent radiative transfer treatment of the dust temperature, which controls much of the chemistry. A small parameter grid is explored to understand the effects of the sound speed and the mass and rotation of the cloud. The freeze-out and evaporation of carbon monoxide (CO) and water (H2O), as well as the potential for forming complex organic molecules in ices, are considered as important first steps to illustrate the full chemistry. Results. Both species freeze out towards the centre before the collapse begins. Pure CO ice evaporates during the infall phase and re-adsorbs in those parts of the disk that cool below the CO desorption temperature of ~18 K. H2O remains solid almost everywhere during the infall and disk formation phases and evaporates within ~10 AU of the star. Mixed CO-H2O ices are important in keeping some solid CO above 18 K and in explaining the presence of CO in comets. Material that ends up in the planet- and comet-forming zones of the disk is predicted to spend enough time in a warm zone during the collapse to form first-generation complex organic species on the grains. The dynamical timescales in the hot inner envelope (hot core or hot corino) are too short for abundant formation of second-generation molecules by high-temperature gas-phase chemistry.

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R. Visser, E. F. van Dishoeck, S. D. Doty, C. P. Dullemond. 2009-01-09. The chemical history of molecules in circumstellar disks. I. Ices. https://doi.org/10.1051/0004-6361%2F200810846

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