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arXiv · 0909.1756

Atomic carbon chains as spin-transmitters: an \textit{Ab initio} transport study

Joachim A. Fuerst·Mads Brandbyge·Antti-Pekka Jauho
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Abstract

An atomic carbon chain joining two graphene flakes was recently realized in a ground-breaking experiment by Jin {\it et al.}, Phys. Rev. Lett. {\bf 102}, 205501 (2009). We present {\it ab initio} results for the electron transport properties of such chains and demonstrate complete spin-polarization of the transmission in large energy ranges. The effect is due to the spin-polarized zig-zag edge terminating each graphene flake causing a spin-splitting of the graphene $π_z$ bands, and the chain states. Transmission occurs when the graphene $π$-states resonate with similar states in the strongly hybridized edges and chain. This effect should in general hold for any $π$-conjugated molecules bridging the zig-zag edges of graphene electrodes. The polarization of the transmission can be controlled by chemically or mechanically modifying the molecule, or by applying an electrical gate.

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Joachim A. Fuerst, Mads Brandbyge, Antti-Pekka Jauho. 2010-06-17. Atomic carbon chains as spin-transmitters: an \textit{Ab initio} transport study. https://doi.org/10.1209/0295-5075%2F91%2F37002

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