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arXiv · 1001.2601

Pressure-induced new magnetic phase in Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ probed by muon spin rotation

Takao Suzuki·Isao Watanabe·Fumiko Yamada·Motoki Yamada·Yasuyuki Ishii·Takayuki Kawamata·Takayuki Goto·Hidekazu Tanaka
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Abstract

We carried out zero-field muon-spin-rotation (ZF-$μ$SR) measurements in hydrostatic pressures in impurity-doped quantum spin gap system Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ to investigate microscopic magnetic properties of the pressure-induced phase. The spontaneous muon spin precession, which indicates the existence of a long-range coherent order, is observed in pressures. With decreasing temperature in 3.1 kbar, the internal static magnetic field at the muon sites {\it H}$_{\rm int}$ tends to saturate to 280 Oe around 4 K, however, decreases to 240 Oe at 2.3 K. These results suggest a rearrangement of ordered spins, and we speculate that the oblique antiferromagnetic phase, which is observed in the pressure of 14 kbar on the pure TlCuCl$_3$, appears in the Mg-doped system in lower pressures.

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Takao Suzuki, Isao Watanabe, Fumiko Yamada, Motoki Yamada, Yasuyuki Ishii, Takayuki Kawamata, Takayuki Goto, Hidekazu Tanaka. 2010-01-15. Pressure-induced new magnetic phase in Tl(Cu$_{0.985}$Mg$_{0.015}$)Cl$_3$ probed by muon spin rotation. https://doi.org/10.1088/1742-6596%2F225%2F1%2F012054

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