Defects in Heavy-Fermion Materials: Unveiling Strong Correlations in Real Space

Abstract

Complexity in materials often arises from competing interactions at the atomic length scale. One such example are the strongly correlated heavy-fermion materials where the competition between Kondo screening and antiferromagnetic ordering is believed to be the origin of their puzzling non-Fermi-liquid properties. Insight into such complex physical behavior in strongly correlated electron systems can be gained by impurity doping. Here, we develop a microscopic theoretical framework to demonstrate that defects implanted in heavy-fermion materials provide an opportunity for unveiling competing interactions and their correlations in real space. Defect-induced perturbations in the electronic and magnetic correlations possess characteristically different spatial patterns that can be visualized via their spectroscopic signatures in the local density of states or non-local spin susceptibility. These real space patterns provide insight into the complex electronic structure of heavy-fermion materials, the light or heavy character of the perturbed states, and the hybridization between them. The strongly correlated nature of these materials also manifests itself in highly non-linear quantum interference effects between defects that can drive the system through a first-order phase transition to a novel inhomogeneous ground state.