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arXiv · 1002.0920

Near-infrared single-photons from aligned molecules in ultrathin crystalline films at room temperature

C. Toninelli·K. Early·J. Bremi·A. Renn·S. Goetzinger·V. Sandoghdar
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Abstract

We investigate the optical properties of Dibenzoterrylene (DBT) molecules in a spin-coated crystalline film of anthracence. By performing single molecule studies, we show that the dipole moments of the DBT molecules are oriented parallel to the plane of the film. Despite a film thickness of only 20 nm, we observe an exceptional photostability at room temperature and photon count rates around one million per second from a single molecule. These properties together with an emission wavelength around 800 nm make this system attractive for applications in nanophotonics and quantum optics.

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C. Toninelli, K. Early, J. Bremi, A. Renn, S. Goetzinger, V. Sandoghdar. 2010-02-04. Near-infrared single-photons from aligned molecules in ultrathin crystalline films at room temperature. https://doi.org/10.1364/oe.18.006577

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