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arXiv · 1204.6210

Coupling of spin and lattice modes in the S=1/2 two-dimensional antiferromagnet K$_{2}$V$_{3}$O$_{8}$ with magneto-dielectric couplings

K. -Y. Choi·P. Lemmens·V. P. Gnezdilov·B. C. Sales·M. D. Lumsden
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Abstract

Lattice dynamics and magnetic excitations are investigated to elucidate the origin of magneto-dielectric effects in the S=1/2 two-dimensional quantum spin compound K$_2$V$_3$O$_8$. We find evidence for lattice instabilities at 110 K and 60 K as optical phonon anomalies and a soft mode at 26 cm$^{-1}$ in A$_1$ symmetry. Two-magnon excitations in B$_1$ symmetry show an unconventional double-peak structure and temperature dependence. This suggests the existence of a split mode near the zone boundary caused by a mixing of spin and lattice modes.

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K. -Y. Choi, P. Lemmens, V. P. Gnezdilov, B. C. Sales, M. D. Lumsden. 2012-04-27. Coupling of spin and lattice modes in the S=1/2 two-dimensional antiferromagnet K$_{2}$V$_{3}$O$_{8}$ with magneto-dielectric couplings. https://doi.org/10.1103/physrevb.85.144434

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