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arXiv · 1206.4913

Magnetic Order and Fluctuations in the Presence of Quenched Disorder in the Kagome Staircase System (Co(1-x)Mg(x))3V2O8

Katharina Fritsch·Zahra Yamani·Sung Chang·Yiming Qiu·John R. D. Copley·Mehmet Ramazanoglu·Hanna A. Dabkowska·Bruce D. Gaulin
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Abstract

Co3V2O8 is an orthorhombic magnet in which S=3/2 magnetic moments reside on two crystallographically inequivalent Co2+ sites, which decorate a stacked, buckled version of the two dimensional kagome lattice, the stacked kagome staircase. The magnetic interactions between the Co2+ moments in this structure lead to a complex magnetic phase diagram at low temperature, wherein it exhibits a series of five transitions below 11 K that ultimately culminate in a simple ferromagnetic ground state below T~6.2 K. Here we report magnetization measurements on single and polycrystalline samples of (Co(1-x)Mg(x))3V2O8 for x<0.23, as well as elastic and inelastic neutron scattering measurements on single crystals of magnetically dilute (Co(1-x)Mg(x))3V2O8 for x=0.029 and x=0.194, in which non-magnetic Mg2+ ions substitute for magnetic Co2+. We find that a dilution of 2.9% leads to a suppression of the ferromagnetic transition temperature by ~15% while a dilution level of 19.4% is sufficient to destroy ferromagnetic long-range order in this material down to a temperature of at least 1.5 K. The magnetic excitation spectrum is characterized by two spin-wave branches in the ordered phase for (Co(1-x)Mg(x))3V2O8 (x=0.029), similar to that of the pure x=0 material, and by broad diffuse scattering at temperatures below 10 K in (Co(1-x)Mg(x))3V2O8 (x=0.194). Such a strong dependence of the transition temperatures to long range order in the presence of quenched non-magnetic impurities is consistent with two-dimensional physics driving the transitions. We further provide a simple percolation model that semi-quantitatively explains the inability of this system to establish long-range magnetic order at the unusually-low dilution levels which we observe in our experiments.

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Katharina Fritsch, Zahra Yamani, Sung Chang, Yiming Qiu, John R. D. Copley, Mehmet Ramazanoglu, Hanna A. Dabkowska, Bruce D. Gaulin. 2012-06-21. Magnetic Order and Fluctuations in the Presence of Quenched Disorder in the Kagome Staircase System (Co(1-x)Mg(x))3V2O8. https://doi.org/10.1103/physrevb.86.174421

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