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arXiv · 1208.5921

Asymmetric Thermal Lineshape Broadening in a Gapped 3-Dimensional Antiferromagnet - Evidence for Strong Correlations at Finite Temperature

D. L. Quintero-Castro·B. Lake·A. T. M. N. Islam·E. M. Wheeler·C. Balz·M. Mansson·K. C. Rule·S. Gvasaliya·A. Zheludev
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Abstract

It is widely believed that magnetic excitations become increasingly incoherent as temperature is raised due to random collisions which limit their lifetime. This picture is based on spin-wave calculations for gapless magnets in 2 and 3 dimensions and is observed experimentally as a symmetric Lorentzian broadening in energy. Here, we investigate a three-dimensional dimer antiferromagnet and find unexpectedly that the broadening is asymmetric - indicating that far from thermal decoherence, the excitations behave collectively like a strongly correlated gas. This result suggests that a temperature activated coherent state of quasi-particles is not confined to special cases like the highly dimerized spin-1/2 chain but is found generally in dimerized antiferromagnets of all dimensionalities and perhaps gapped magnets in general.

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D. L. Quintero-Castro, B. Lake, A. T. M. N. Islam, E. M. Wheeler, C. Balz, M. Mansson, K. C. Rule, S. Gvasaliya, A. Zheludev. 2012-08-29. Asymmetric Thermal Lineshape Broadening in a Gapped 3-Dimensional Antiferromagnet - Evidence for Strong Correlations at Finite Temperature. https://doi.org/10.1103/physrevlett.109.127206

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