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arXiv · 1209.5100

On the Origin of Zigzag Magnetic Order in Iridium Oxide Na2IrO3

Jiří Chaloupka·George Jackeli·Giniyat Khaliullin
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Abstract

We explore the phase diagram of spin-orbit Mott insulators on a honeycomb lattice, within the Kitaev-Heisenberg model extended to its full parameter space. Zigzag-type magnetic order is found to occupy a large part of the phase diagram of the model, and its physical origin is explained as due to interorbital t2g-eg hopping. Magnetic susceptibility and spin wave spectra are calculated and compared to the experimental data, obtaining thereby the spin coupling constants in Na2IrO3 and Li2IrO3.

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Jiří Chaloupka, George Jackeli, Giniyat Khaliullin. 2012-09-23. On the Origin of Zigzag Magnetic Order in Iridium Oxide Na2IrO3. https://doi.org/10.1103/physrevlett.110.097204

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