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arXiv · 1212.3667

Fabrication of CeO2 by sol-gel process based on microfluidic technology as an analog preparation of ceramic nuclear fuel microspheres

Bin Ye·Jilang Miao·Jiaolong Li·Zichen Zhao·Zhenqi Chang·Christophe A. Serra
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Abstract

Microfluidics integrated with sol-gel processes is introduced in preparing monodispersed MOX nuclear fuel microspheres using nonactive cerium as a surrogate for uranium or plutonium. The detailed information about microfluidic devices and sol-gel processes are provided. The effects of viscosity and flow rate of continuous and dispersed phase on size and size distribution of CeO2 microspheres have been investigated. A comprehensive characterization of the CeO2 microspheres has been conducted, including XRD pattern, SEM, density, size and size distribution. The size of prepared monodisperse particles can be controlled precisely in range of 10{\mu}m to 1000{\mu}m and the particle CV is below 3%.

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Bin Ye, Jilang Miao, Jiaolong Li, Zichen Zhao, Zhenqi Chang, Christophe A. Serra. 2012-12-15. Fabrication of CeO2 by sol-gel process based on microfluidic technology as an analog preparation of ceramic nuclear fuel microspheres. https://doi.org/10.1080/00223131.2013.796897

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