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arXiv · 1301.5056

Quasi-two-dimensional non-collinear magnetism in the Mott insulator Sr$_2$F$_2$Fe$_2$OS$_2$

Liang L. Zhao·Shan Wu·Jiakui K. Wang·J. P. Hodges·C. Broholm·E. Morosan
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Abstract

The magnetism of Sr$_2$F$_2$Fe$_2$OS$_2$ was examined through neutron powder diffraction and thermodynamic and transport measurements. Quasi-two-dimensional magnetic order develops below $T_N$ = 106(2) K with an in-plane correlation length exceeding 310 Å and an out-of-plane correlation length of just 17(3) Å. The data are consistent with a two-k structure with $k_1$ = (1/2, 0, 1/2) and $k_2$ = (0, 1/2, 1/2) and an ordered moment of 3.3(1) $μ_B$ oriented along the in-plane components of k. This structure is composed of orthogonal AFM chains intersecting at super-exchange mediating O sites. Density Functional Theory (DFT) also points to this structure and a narrower Fe 3d band than for the iron pnictides from which electronic correlations produce a Mott insulator.

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Liang L. Zhao, Shan Wu, Jiakui K. Wang, J. P. Hodges, C. Broholm, E. Morosan. 2013-01-22. Quasi-two-dimensional non-collinear magnetism in the Mott insulator Sr$_2$F$_2$Fe$_2$OS$_2$. https://doi.org/10.1103/physrevb.87.020406

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