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arXiv · 1303.1362

High-order harmonic generation from field-distorted orbitals

Maciej Dominik Śpiewanowski·Adam Etches·Lars Bojer Madsen
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Abstract

We investigate the effect on high-order harmonic generation of the distortion of molecular orbitals by the driving laser field. Calculations for high-order harmonic generation including orbital distortion are performed for N2. Our results allow us to suggest that field-distortion is the reason why the two-center interference minimum has never been observed experimentally in N2. We propose experimental parameters which should allow an observation of the two-center interference minimum.

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Maciej Dominik Śpiewanowski, Adam Etches, Lars Bojer Madsen. 2013-03-06. High-order harmonic generation from field-distorted orbitals. https://doi.org/10.1103/physreva.87.043424

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