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arXiv · 1303.7265

Microscopic and Spectroscopic Evidence for a Slater Metal-Insulator Transition in Sr2IrO4

Qing Li·Guixin Cao·Satoshi Okamoto·Jieyu Yi·Wenzhi Lin·Brian C. Sales·Jiaqiang Yan·Ryotaro Arita·Jan Kunes·Anton V. Kozhevnikov·Adolfo G. Eguiluz·Masatoshi Imada·Zheng Gai·Minghu Pan·David G. Mandrus
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Abstract

Layered 5d transition metal oxides (TMOs) have attracted significant interest in recent years because of the rich physical properties induced by the interplay between spin-orbit coupling, bandwidth and on-site Coulomb repulsion. In Sr2IrO4, this interplay opens a gap near the Fermi energy and stabilizes a Jeff=1/2 spin-orbital entangled insulating state at low temperatures. Whether this metal-insulating transition (MIT) is Mott-type (electronic-correlation driven) or Slater-type (magnetic-order driven) has been under intense debate. We address this issue via spatially resolved imaging and spectroscopic studies of the Sr2IrO4 surface using scanning tunneling microscopy/spectroscopy (STM/S). The STS results clearly illustrate the opening of the (~150-250 meV) insulating gap at low temperatures, in qualitative agreement with our density-functional theory (DFT) calculations. More importantly, the measured temperature dependence of the gap width coupled with our DFT+dynamical mean field theory (DMFT) results strongly support the Slater-type MIT scenario in Sr2IrO4. The STS data further reveal a pseudogap structure above the Neel temperature, presumably related to the presence of antiferromagnetic fluctuations.

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Qing Li, Guixin Cao, Satoshi Okamoto, Jieyu Yi, Wenzhi Lin, Brian C. Sales, Jiaqiang Yan, Ryotaro Arita, Jan Kunes, Anton V. Kozhevnikov, Adolfo G. Eguiluz, Masatoshi Imada, Zheng Gai, Minghu Pan, David G. Mandrus. 2013-03-28. Microscopic and Spectroscopic Evidence for a Slater Metal-Insulator Transition in Sr2IrO4. https://arxiv.org/abs/1303.7265

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