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arXiv · 1307.4871

Magnetic properties of La(0.67)Sr(0.33)MnO3/BiFeO3(001) heterojunctions: chemically abrupt versus atomic intermixed interface

R. F. Neumann·M. Bahiana·N. Binggeli
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Abstract

Using first-principles density-functional calculations, we address the magnetic properties of the ferromagnet/antiferromagnet La(0.67)Sr(0.33)MnO3/BiFeO3(001) heterojunctions, and investigate possible driving mechanisms for a ferromagnetic (FM) interfacial ordering of the Fe spins recently observed experimentally. We find that the chemically abrupt defect-free La(0.67)Sr(0.33)MnO3/BiFeO3(001) heterojunction displays, as ground state, an ordering with compensated Fe spins. Cation Fe/Mn intermixing at the interface tends to favour, instead, a FM interfacial order of the Fe spins, coupled antiferromagnetically to the bulk La(0.67)Sr(0.33)MnO3 spins, as observed experimentally. Such trends are understood based on a model description of the energetics of the exchange interactions.

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R. F. Neumann, M. Bahiana, N. Binggeli. 2013-07-18. Magnetic properties of La(0.67)Sr(0.33)MnO3/BiFeO3(001) heterojunctions: chemically abrupt versus atomic intermixed interface. https://doi.org/10.1209/0295-5075%2F100%2F67002

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