Ground-state magnetic phase diagram of bow-tie graphene nanoflakes in external magnetic field

Karol Szałowski

doi:10.1063/1.4858378

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arXiv · 1312.7298

Ground-state magnetic phase diagram of bow-tie graphene nanoflakes in external magnetic field

Karol Szałowski

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Abstract

The magnetic phase diagram of a ground state is studied theoretically for graphene nanoflakes of bow-tie shape and various size in external in-plane magnetic field. The tight-binding Hamiltonian supplemented with Hubbard term is used to model the electronic structure of the systems in question. The existence of the antiferromagnetic phase with magnetic moments localized at the sides of the bow-tie is found for low field and a field-induced spin-flip transition to ferromagnetic state is predicted to occur in charge-undoped structures. For small nanoflake doped with a single charge carrier the low-field phase is ferrimagnetic and a metamagnetic transition to ferromagnetic ordering can be forced by the field. The critical field is found to decrease with increasing size of the nanoflake. The influence of diagonal and off-diagonal disorder on the mentioned magnetic properties is studied. The effect of off-diagonal disorder is found to be more important than this of diagonal disorder, leading to significantly widened distribution of critical fields for disordered population of nanoflakes.

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Karol Szałowski. 2013-12-27. Ground-state magnetic phase diagram of bow-tie graphene nanoflakes in external magnetic field. https://doi.org/10.1063/1.4858378

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