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arXiv · 1403.0208

Spin disorder in an Ising honeycomb chain cobaltate

Hirokazu Igarashi·Yasuhiro Shimizu·Yoshiaki Kobayashi·Masayuki Itoh
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Abstract

We report on a member of the spin-disordered honeycomb lattice antiferromagnet in a quasi-one-dimensional cobaltate Ba_3Co_2O_6(CO_3)_0.7. Resistivity exhibits as semimetallic along the face-sharing CoO6 chains. Magnetic susceptibility shows strongly anisotropic Ising-spin character with the easy axis along the chain due to significant spin-orbit coupling and a trigonal crystal field. Nevertheless, ^135Ba NMR detects no indication of the long-range magnetic order down to 0.48 K. Marginally itinerant electrons possess large entropy and low-lying excitations with a Wilson ratio R_W = 116, which highlight interplays of charge, spin, and orbital in the disordered ground state.

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Hirokazu Igarashi, Yasuhiro Shimizu, Yoshiaki Kobayashi, Masayuki Itoh. 2014-03-02. Spin disorder in an Ising honeycomb chain cobaltate. https://doi.org/10.1103/physrevb.89.054431

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