Nonlinear Doppler - Free comb-spectroscopy in counter-propagating fields

Abstract

The method of Doppler - free comb - spectroscopy for dipole transitions was proposed. The calculations for susceptibility spectrum for moving two-level atoms driving by strong counter propagating combs have been done. The used theoretical method based on the Fourier expansion of the components of density matrix on two rows on kv (v-velocity of group of atoms, k-projection of wave vector) and {\Omega} (frequency between comb components). For testing of validity of this method the direct numerical integration was done. The narrow peaks with homogeneous width arise on the background of Doppler counter. The contrast of these peaks is large for largest amplitudes of comb-components. Power broadening is increasing with increase of field amplitudes. The spectral range of absorption spectrum is determined by the spectral range of comb generator and all homogeneous lines arise simultaneously. The spectral resolution is determined by the width of homogeneously-broadening lines. The physical nature of narrow peaks is in the existence of multi-photon transitions between manifolds of quasi-energy levels arising for different groups of atoms moving with velocities that satisfy to the resonant conditions 2kv= (n+l){\Omega}, where n, l - are integers and {\Omega} - frequency difference between comb teeth.