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arXiv · 1404.0044

Nonmagnetic ordering state of single-crystal SrTm$_2$O$_4$: A polarized and unpolarized neutron-scattering study

Haifeng Li·Binyang Hou·Andrew Wildes·Anatoliy Senyshyn·Karin Schmalzl·Wolfgang Schmidt·Cong Zhang·Thomas Brueckel·Georg Roth
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Abstract

Our single-crystal polarized neutron scattering at 65 mK and powder unpolarized neutron diffraction at 0.5 K show no evidence for a long-range magnetic order and even detect no sign of diffuse magnetic neutron scattering in single-crystal SrTm2O4. The data refinements reveal that the two TmO6 octahedral distortion modes are the same as those of the TbO6 octahedra in SrTb2O4, i.e., one distortion is stronger than the other one especially at low temperatures, which is attributed probably to different crystal electric fields for the two inequivalent octahedra. Consequently, we conclude that SrTm2O4 has no magnetic order, neither long-ranged nor short-ranged, even down to 65 mK. Therefore, SrTm2O4 is a different compound from its brethren in the new family of frustrated SrRE2O4 (RE = Gd, Tb, Dy, Ho, Er, and Yb) magnets. We propose that crystal field anisotropy may dominate over weak dipolar spin interactions in SrTm2O4, leading to a virtually nonmagnetic ordering state.

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Haifeng Li, Binyang Hou, Andrew Wildes, Anatoliy Senyshyn, Karin Schmalzl, Wolfgang Schmidt, Cong Zhang, Thomas Brueckel, Georg Roth. 2014-03-31. Nonmagnetic ordering state of single-crystal SrTm$_2$O$_4$: A polarized and unpolarized neutron-scattering study. https://doi.org/10.1039/c5tc01607j

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