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arXiv · 1409.1591

Correlating Quasi-Electron Relaxation with Quantum Femtosecond Magnetism in the Order Parameter Dynamics of Insulating Manganites

T. Li·A. Patz·P. Lingos·L. Mouchliadis·L. Li·J. Yan·I. E. Perakis·J. Wang
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Abstract

Femtosecond (fs)-resolved simultaneous measurements of charge and spin dynamics reveal the coexistence of two different quasi-particle excitations in colossal magneto-resistive (CMR) manganites, with {\em fs} and {\em ps} relaxation times respectively. Their populations reverse size above a {\em photoexcitation-intensity-threshold} coinciding with a "sudden" antiferro-to-ferromagnetic switching during $<$100 fs laser pulses. We present evidence that fast, metallic, mobile quasi--electrons dressed by {\em quantum spin fluctuations} coexist with slow, localized, polaronic charge carriers in non-equilibrium phases. This may be central to CMR transition and leads to a laser-driven charge reorganization simultaneously with quantum fs magnetism via an emergent quantum-spin/charge/lattice transient coupling.

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T. Li, A. Patz, P. Lingos, L. Mouchliadis, L. Li, J. Yan, I. E. Perakis, J. Wang. 2014-09-03. Correlating Quasi-Electron Relaxation with Quantum Femtosecond Magnetism in the Order Parameter Dynamics of Insulating Manganites. https://doi.org/10.1103/physrevb.95.224432

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