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arXiv · 1410.6459

Spin-orbiton and quantum criticality in FeSc2S4

L. Mittelstädt·M. Schmidt·Zhe Wang·F. Mayr·V. Tsurkan·P. Lunkenheimer·D. Ish·L. Balents·J. Deisenhofer·A. Loidl
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Abstract

In FeSc2S4 spin-orbital exchange competes with strong spin-orbit coupling, suppressing long-range spin and orbital order and, hence, this material represents one of the rare examples of a spin-orbital liquid ground state. Moreover, it is close to a quantum-critical point separating the ordered and disordered regimes. Using THz and FIR spectroscopy we study low-lying excitations in FeSc2S4 and provide clear evidence for a spin-orbiton, an excitation of strongly entangled spins and orbitals. It becomes particularly well pronounced upon cooling, when advancing deep into the quantum-critical regime. Moreover, indications of an underlying structureless excitation continuum are found, a possible signature of quantum criticality.

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L. Mittelstädt, M. Schmidt, Zhe Wang, F. Mayr, V. Tsurkan, P. Lunkenheimer, D. Ish, L. Balents, J. Deisenhofer, A. Loidl. 2015-01-22. Spin-orbiton and quantum criticality in FeSc2S4. https://doi.org/10.1103/physrevb.91.125112

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