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arXiv · 1502.00057

Spontaneous multipole ordering by local parity mixing

Satoru Hayami·Hiroaki Kusunose·Yukitoshi Motome
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Abstract

Broken spatial inversion symmetry in spin-orbital coupled systems leads to a mixing between orbitals with different parity, which results in unusual electronic structures and transport properties. We theoretically investigate the possibility of multipole ordering induced by a parity mixing. In particular, we focus on the system in which the parity mixing appears in a sublattice-dependent form. Starting from the periodic Anderson model with such a local parity mixing, we derive an extended Kondo lattice model with sublattice-dependent antisymmetric exchange couplings between itinerant electrons and localized spins. By the variational calculation, simulated annealing, and Monte Carlo simulation, we show that the model on a quasi-one-dimensional zig-zag lattice exhibits an odd-parity multipole order composed of magnetic toroidal and quadrupole components at and near half filling. The multipole order causes a band deformation with the band bottom shift and a magnetoelectric response. The results suggest that unusual odd-parity multipole orders will be widely observed in multi-orbital systems with local parity mixing.

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Satoru Hayami, Hiroaki Kusunose, Yukitoshi Motome. 2015-01-31. Spontaneous multipole ordering by local parity mixing. https://doi.org/10.7566/jpsj.84.064717

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