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arXiv · 1503.03106

Negative-Temperature State Formed and Interactions Inverted by Symmetric Monocycle Optical Pulse Excitation

Kenji Yonemitsu·Keita Nishioka
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Abstract

The excited state dynamics of correlated electron and electron-phonon systems triggered by an oscillating electric-field pulse of large amplitude are theoretically investigated. A "negative-temperature" state and inversion of electron-electron and electron-phonon interactions are induced even by a symmetric monocycle pulse. This fact is numerically demonstrated, using the exact diagonalization method, in a band-insulator phase of one-dimensional three-quarter-filled strongly dimerized extended Peierls-Hubbard and Holstein models. When the total-energy increment is maximized as a function of the electric field amplitude, the occupancy of the bonding and antibonding orbitals is inverted to produce a negative-temperature state. Around this state, the dependences of time-averaged electron-electron and electron-phonon correlation functions on interaction parameters are opposite to those in the ground state.

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Kenji Yonemitsu, Keita Nishioka. 2015-03-10. Negative-Temperature State Formed and Interactions Inverted by Symmetric Monocycle Optical Pulse Excitation. https://doi.org/10.7566/jpsj.84.054702

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