Evolution of quasiparticle excitations with critical mass enhancement in superconducting AFe2As2 (A = K, Rb, and Cs)

Abstract

In the heavily hole-doped iron-based superconductors $A$Fe$_2$As$_2$ ($A=$ K, Rb, and Cs), the electron effective mass increases rapidly with alkali-ion radius. To study how the mass enhancement affects the superconducting state, we measure the London penetration depth $λ(T)$ in clean crystals of $A$Fe$_2$As$_2$ down to low temperature $T\sim0.1$ K. In all systems, the superfluid stiffness $ρ_s(T)=λ^2(0)/λ^2(T)$ can be approximated by a power-law $T$ dependence at low temperatures, indicating the robustness of strong momentum anisotropy in the superconducting gap $Δ(k)$. The power $α$ increases from $\sim1$ with mass enhancement and approaches an unconventional exponent $α\sim 1.5$ in the heaviest CsFe$_2$As$_2$. This appears to be a hallmark of superconductors near antiferromagnetic quantum critical points, where the quasiparticles excited across the anisotropic $Δ(k)$ are significantly influenced by the momentum dependence of quantum critical fluctuations.