Towards the full quantum dynamical description of photon induced processes in $\mathrm{D}_{2}^{+}$

Attila Tóth; Sándor Borbély; Zsolt G. Kiss; Gábor J. Halász; Ágnes Vibók

doi:10.1021/acs.jpca.6b09623

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arXiv · 1601.05374

Towards the full quantum dynamical description of photon induced processes in $\mathrm{D}_{2}^{+}$

Attila Tóth·Sándor Borbély·Zsolt G. Kiss·Gábor J. Halász·Ágnes Vibók

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Abstract

A new quantum dynamical model has been developed to describe the dissociative ionization of deuterium molecular ions by intense laser pulses ($τ=10$ fs, $λ=200$ nm and $I=3\times10^{13}$ W/cm$^{2}$). We calculated the ionization probability densities by solving the time-dependent Schrödinger equation numerically. Throughout the simulation the nuclear vibration was considered as a dynamic variable with fixed molecular axis orientation. Benchmark calculations were performed for the ionization of $\mathrm{HeH}^{++}$, for which accurate numerical results are available in the literature, in order to check the performance of this new restricted model.

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Attila Tóth, Sándor Borbély, Zsolt G. Kiss, Gábor J. Halász, Ágnes Vibók. 2016-01-20. Towards the full quantum dynamical description of photon induced processes in $\mathrm{D}_{2}^{+}$. https://doi.org/10.1021/acs.jpca.6b09623

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