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arXiv · 1603.02043

Site-specific $^{13}$C NMR study on locally distorted triangular lattice of organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$

Y. Saito·T. Minamidate·A. Kawamoto·N. Matsunaga·K. Nomura
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Abstract

To verify the effect of geometrical frustration, we artificially distort the triangular lattice of quasi-two-dimensional organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ [BEDT-TTF: bis(ethylenedithio)terathiofulvalene] by analogous-molecular substitution and apply $^{13}$C NMR of bulk and substituted sites, electric conductivity, and static magnetic susceptibility measurements. The results indicate that the magnetic characteristics of the substituted sample are quantitatively similar to those of the pure sample. Moreover the magnetic characteristics at the substituted sites are also the same as in the bulk. These results suggest that the observed magnetic properties may not be due to the geometrical frustration but the importance of disorder.

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Y. Saito, T. Minamidate, A. Kawamoto, N. Matsunaga, K. Nomura. 2016-03-07. Site-specific $^{13}$C NMR study on locally distorted triangular lattice of organic conductor $\kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$. https://doi.org/10.1103/physrevb.98.205141

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