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arXiv · 1604.07747

Modulated spin helicity stabilized by incommensurate orbital density waves in a quadruple perovskite manganite

R. D. Johnson·D. D. Khalyavin·P. Manuel·A. Bombardi·C. Martin·L. C. Chapon·P. G. Radaelli
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Abstract

Through a combination of neutron diffraction and Landau theory we describe the spin ordering in the ground state of the quadruple perovskite manganite CaMn7O12 - a magnetic multiferroic supporting an incommensurate orbital density wave that onsets above the magnetic ordering temperature, TN1 = 90 K. The multi-k magnetic structure in the ground state was found to be a nearly-constant-moment helix with modulated spin helicity, which oscillates in phase with the orbital occupancies on the Mn3+ sites via trilinear magneto-orbital coupling. Our phenomenological model also shows that, above TN2 = 48 K, the primary magnetic order parameter is locked into the orbital wave by an admixture of helical and collinear spin density wave structures. Furthermore, our model naturally explains the lack of a sharp dielectric anomaly at TN1 and the unusual temperature dependence of the electrical polarisation.

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R. D. Johnson, D. D. Khalyavin, P. Manuel, A. Bombardi, C. Martin, L. C. Chapon, P. G. Radaelli. 2016-04-26. Modulated spin helicity stabilized by incommensurate orbital density waves in a quadruple perovskite manganite. https://doi.org/10.1103/physrevb.93.180403

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