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arXiv · 1702.06687

Origin of luminescence quenching in structures containing CdSe/ZnSe quantum dots with a few Mn$^{2+}$ ions

Kacper Oreszczuk·Mateusz Goryca·Wojciech Pacuski·Tomasz Smoleński·Michał Nawrocki·Piotr Kossacki
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Abstract

We present a detailed spectroscopic study of the photoluminescence quenching in an epitaxial structures containing CdSe/ZnSe quantum dots doped with low concentration of Mn$^{2+}$ ions. Our time-resolved and time-integrated experiments reveal the origin of the quenching observed in macro-photoluminescence studies of ensembles of such dots. We show that incorporation of even a few ions to an individual dot does not quench its luminescence effectively, although some fingerprints of expected spin-dependent quenching are visible. At the same time, the presence of Mn$^{2+}$ ions in the sample significantly affects the luminescence intensity of the wetting layer, resulting in a quenching of the global luminescence from studied structure. On the other hand, the luminescence decay dynamics is found to be independent of the presence of Mn$^{2+}$ ions, which suggests that the observed quenching occurs for the excited excitonic states.

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Kacper Oreszczuk, Mateusz Goryca, Wojciech Pacuski, Tomasz Smoleński, Michał Nawrocki, Piotr Kossacki. 2017-11-09. Origin of luminescence quenching in structures containing CdSe/ZnSe quantum dots with a few Mn$^{2+}$ ions. https://doi.org/10.1103/physrevb.96.205436

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