Doppler-free resolution near-infrared spectroscopy at 1.28~$μ$m with the noise-immune cavity-enhanced optical heterodyne molecular spectroscopy method

Abstract

We report on the Doppler-free saturation spectroscopy of the nitrous oxide (N$_2$O) overtone transition at 1.28~$μ$m. This measurement is performed by the noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS) technique based on the quantum-dot (QD) laser. A high intra-cavity power, up to 10~W, reaches the saturation limit of the overtone line using an optical cavity with a high finesse of 113,500. At a pressure of several mTorr, the saturation dip is observed with a full width at half-maximum of about 2~MHz and a signal-to-noise ratio of 71. To the best of our knowledge, this is the first saturation spectroscopy of molecular overtone transitions in 1.3~$μ$m region. The QD laser is then locked to this dispersion signal with a stability of 15 kHz at 1 sec integration time. We demonstrate the potential of the N$_2$O as markers because of its particularly rich spectrum at the vicinity of 1.28-1.30 $μ$m where lies several important forbidden transitions of atomic parity violation measurements and the 1.3 $μ$m O-band of optical communication.