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arXiv · 1706.02872

Low Curie-temperature ferromagnetic phase in SmPt2Cd20 possibly accompanied by strong quantum fluctuations

Akira Yamada·Shota Oike·Ryuji Higashinaka·Tatsuma D. Matsuda·Yuji Aoki
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Abstract

Electrical resistivity, magnetization and specific heat have been measured for single crystals of SmPt$_{2}$Cd$_{20}$. It has been found that SmPt$_{2}$Cd$_{20}$ exhibits a ferromagnetic (FM) transition at $T_{\rm C} = 0.64$ K, the lowest among cubic compounds. Specific heat divided by temperature increases with decreasing temperature even below $T_{\rm C}$ and attains 4.5 J/mol K$^{2}$ at 0.26 K, implying substantial magnetic quantum fluctuations. An analysis of the magnetic entropy suggests the crystalline-electric-field splitting of the Sm $J = 5/2$ multiplet with a $Γ_{7}$ doublet ground state and a $Γ_8$ quartet excited state (the excitation energy of $\sim30$ K). The electrical resistivity shows a power-law behavior with $T^{0.74}$ below 2 K without showing any noticeable anomaly at $T_{\rm C}$. SmPt$_{2}$Cd$_{20}$ is regarded as a rare cubic system that is located in the vicinity of a FM quantum critical point.

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Akira Yamada, Shota Oike, Ryuji Higashinaka, Tatsuma D. Matsuda, Yuji Aoki. 2017-06-09. Low Curie-temperature ferromagnetic phase in SmPt2Cd20 possibly accompanied by strong quantum fluctuations. https://doi.org/10.1103/physrevb.96.085102

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