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arXiv · 1805.02271

Resonant thermoelectric transport in atomic chains with Fano defects

J. Eduardo González·Vicenta Sánchez·Chumin Wang
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Abstract

Atomic clusters attached to a low-dimensional system, called Fano defects, produce rich wave interferences. In this work, we analytically found an enhanced thermoelectric figure-of-merit (ZT) in periodic atomic chains with Fano defects, compared to those without such defects. We further study self-assembled DNA-like systems with periodic and quasiperiodically placed Fano defects by using a real-space renormalization method developed for the Kubo-Greenwood formula, in which tight-binding and Born models are respectively used for the electric and lattice thermal conductivities. The results reveal that the quasiperiodicity could be another ZT-improving factor, whose long-range disorder inhibits low-frequency acoustic phonons insensitive to local defects.

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J. Eduardo González, Vicenta Sánchez, Chumin Wang. 2018-05-06. Resonant thermoelectric transport in atomic chains with Fano defects. https://doi.org/10.1557/mrc.2018.84

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