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arXiv · 1809.07526

Turning a molecule into a coherent two-level quantum system

Daqing Wang·Hrishikesh Kelkar·Diego Martin-Cano·Dominik Rattenbacher·Alexey Shkarin·Tobias Utikal·Stephan Götzinger·Vahid Sandoghdar
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Abstract

Molecules are ubiquitous in natural phenomena and man-made products, but their use in quantum optical applications has been hampered by incoherent internal vibrations and other phononic interactions with their environment. We have now succeeded in turning an organic molecule into a coherent two-level quantum system by placing it in an optical microcavity. This allows several unprecedented observations such as 99\% extinction of a laser beam by a single molecule, saturation with less than 0.5 photon, and nonclassical generation of few-photon super-bunched light. Furthermore, we demonstrate efficient interaction of the molecule-microcavity system with single photons generated by a second molecule in a distant laboratory. Our achievements pave the way for linear and nonlinear quantum photonic circuits based on organic platforms.

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Daqing Wang, Hrishikesh Kelkar, Diego Martin-Cano, Dominik Rattenbacher, Alexey Shkarin, Tobias Utikal, Stephan Götzinger, Vahid Sandoghdar. 2018-09-20. Turning a molecule into a coherent two-level quantum system. https://doi.org/10.1038/s41567-019-0436-5

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