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arXiv · 1812.06006

Isospin-phonon coupling and Fano-interference in spin-orbit Mott insulator Sr2IrO4

Kousik Samanta·Danilo Rigitano·Pascoal Jose Giglio Pagliuso·Eduardo Granado
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Abstract

The isospin-phonon coupling in Sr2IrO4 is investigated by temperature dependent phonon Raman scattering. Anomalous behavior in the frequency of all studied optical phonons is observed below the magnetic transition temperature TN ~240 K. The strongest effect is detected for the A1g mode at 272 cm-1 associated with the modulation of the Ir-O-Ir bond angle. Additionally, the A1g mode at 560 cm-1 shows a Fano asymmetric lineshape sensitive to TN, supporting the existence of low-energy (~70 meV) electronic excitations that are renormalized by the magnetic order. These results reveal new aspects of the interaction between the crystal lattice and electronic degrees of freedom in this spin-orbit entangled Mott insulator.

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Kousik Samanta, Danilo Rigitano, Pascoal Jose Giglio Pagliuso, Eduardo Granado. 2018-12-14. Isospin-phonon coupling and Fano-interference in spin-orbit Mott insulator Sr2IrO4. https://doi.org/10.1063/1.5094912

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