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arXiv · 1901.09061

Excitation-assisted nonadiabatic charge-transfer reaction in a mixed atom-ion system

Ming Li·Michael Mills·Prateek Puri·Alexander Petrov·Eric R. Hudson·Svetlana Kotochigova
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Abstract

An important physical process unique to neutral-ion systems is the charge-transfer (CT) reaction. Here, we present measurements of and models for CT processes between co-trapped ultracold Ca atoms and Yb ions under well-controlled conditions. The theoretical analysis reveals the existence of three reaction mechanisms when lasers from a magneto-optical trap (MOT) and an additional catalyst laser are present. Besides the direct CT involving existent excited Ca population in the MOT, the second pathway is controlled by MOT-induced CT, whereas the third one mostly involves the additional red-detuned laser.

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Ming Li, Michael Mills, Prateek Puri, Alexander Petrov, Eric R. Hudson, Svetlana Kotochigova. 2019-01-25. Excitation-assisted nonadiabatic charge-transfer reaction in a mixed atom-ion system. https://doi.org/10.1103/physreva.99.062706

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