arXiv · 1911.05011
Two Coupled Chains are Simpler than One: Field-induced Chirality in a Frustrated Quantum Spin Ladder
Abstract
Although the frustrated spin chain (zigzag chain) is a Drosophila of frustrated magnetism, the understanding of a pair of coupled zigzag chains (frustrated spin ladder) in a magnetic field is incomplete. We address this problem through nuclear magnetic resonance (NMR) experiments on $\text{BiCu}_2\text{PO}_6$ in magnetic fields up to 45 T, revealing a field-induced spiral magnetic structure. Conjointly, we present advanced numerical calculations showing that even moderate rung coupling dramatically simplifies the phase diagram below half-saturation magnetization by stabilizing a field-induced chiral phase. Surprisingly for a one-dimensional model, this phase and its response to Dzyaloshinskii-Moriya (DM) interactions adhere to classical expectations. While explaining the behavior at the highest accessible magnetic fields, our results imply a different origin for the solitonic phases occurring at lower fields in $\text{BiCu}_2\text{PO}_6$. An exciting possibility is that the known, DM-mediated coupling between chirality and crystal lattice gives rise to a new kind of spin-Peierls instability.
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M. Pikulski, T. Shiroka, F. Casola, A. P. Reyes, P. L. Kuhns, S. Wang, H. -R. Ott, J. Mesot. 2019-11-12. Two Coupled Chains are Simpler than One: Field-induced Chirality in a Frustrated Quantum Spin Ladder. https://doi.org/10.1038/s41598-020-72215-z
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