arXiv · 2005.02944
Ignition of a helium nanoplasma by x-ray multiple ionization of a heavy rare-gas core
Abstract
The dynamics of an x-ray-ionized two-component core-shell nanosystem is probed using doped helium (He) nanodroplets. First, a soft x-ray pump pulse selectively inner-shell ionizes the core cluster formed of heavier rare-gas atoms, causing electron migration from the He shell to the highly charged core. This ignites a He nanoplasma which is then driven by an intense near-infrared probe pulse. The ultrafast charge redistribution, evidenced by the rise of He$^+$ and He$^{2+}$ ion yields from the nanoplasma within $<70$ fs, leads to strong damping of the core cluster expansion. Thus, He droplets act as efficient tampers that reduce the radiation damage of embedded nanostructures, a property that could be exploited for improving coherent diffraction images.
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D. Schomas, C. Medina, L. Ben Ltaief, R. B. Fink, S. Mandal, S. R. Krishnan, R. Michiels, M. Debatin, F. Stienkemeier, S. Toleikis, C. Passow, N. Ekanayake, C. Ott, R. Moshammer, T. Pfeifer, A. Heidenreich, M. Mudrich. 2020-05-06. Ignition of a helium nanoplasma by x-ray multiple ionization of a heavy rare-gas core. https://arxiv.org/abs/2005.02944
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