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arXiv · 2008.12203

Ultrafast photocurrents in MoSe$_2$ probed by terahertz spectroscopy

Denis Yagodkin·Lukas Nadvornik·Oliver Gueckstock·Cornelius Gahl·Tobias Kampfrath·Kirill I. Bolotin
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Abstract

We use the terahertz (THz) emission spectroscopy to study femtosecond photocurrent dynamics in the prototypical 2D semiconductor, transition metal dichalcogenide MoSe$_2$. We identify several distinct mechanisms producing THz radiation in response to an ultrashort ($30\,$fs) optical excitation in a bilayer (BL) and a multilayer (ML) sample. In the ML, the THz radiation is generated at a picosecond timescale by out-of-plane currents due to the drift of photoexcited charge carriers in the surface electric field. The BL emission is generated by an in-plane shift current. Finally, we observe oscillations at about $23\,$THz in the emission from the BL sample. We attribute the oscillations to quantum beats between two excitonic states with energetic separation of $\sim100\,$meV.

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Denis Yagodkin, Lukas Nadvornik, Oliver Gueckstock, Cornelius Gahl, Tobias Kampfrath, Kirill I. Bolotin. 2020-12-21. Ultrafast photocurrents in MoSe$_2$ probed by terahertz spectroscopy. https://doi.org/10.1088/2053-1583%2Fabd527

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