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arXiv · 2011.07623

Creation of a novel inverted charge density wave state

Yingchao Zhang·Xun Shi·Mengxue Guan·Wenjing You·Yigui Zhong·Tika R. Kafle·Yaobo Huang·Hong Ding·Michael Bauer·Kai Rossnagel·Sheng Meng·Henry C. Kapteyn·Margaret M. Murnane
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Abstract

Charge density wave (CDW) order is an emergent quantum phase that is characterized by a periodic lattice distortion and charge density modulation, often present near superconducting transitions. Here we uncover a novel inverted CDW state by using a femtosecond laser to coherently over-drive the unique star-of-David lattice distortion in 1T-TaSe$_2$. We track the signature of this novel CDW state using time- and angle-resolved photoemission spectroscopy and time-dependent density functional theory, and validate that it is associated with a unique lattice and charge arrangement never before realized. The dynamic electronic structure further reveals its novel properties, that are characterized by an increased density of states near the Fermi level, high metallicity, and altered electron-phonon couplings. Our results demonstrate how ultrafast lasers can be used to create unique states in materials, by manipulating charge-lattice orders and couplings.

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Yingchao Zhang, Xun Shi, Mengxue Guan, Wenjing You, Yigui Zhong, Tika R. Kafle, Yaobo Huang, Hong Ding, Michael Bauer, Kai Rossnagel, Sheng Meng, Henry C. Kapteyn, Margaret M. Murnane. 2020-11-15. Creation of a novel inverted charge density wave state. https://doi.org/10.1063/4.0000132

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