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arXiv · 2012.15129

Non-equilibrium effects on electron-phonon coupling constant in metals

Wuli Miao·Moran Wang
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Abstract

Understanding of the energy exchange between electrons and phonons in metals is important for micro- and nano-manufacturing and system design. The electron-phonon (e-ph) coupling constant is to describe such exchange strength, yet its variation remains still unclear at micro- and nanoscale where the non-equilibrium effects are significant. In this work, an e-ph coupling model is proposed by transforming the full scattering terms into relaxation time approximation forms in the coupled electron and phonon Boltzmann transport equations. Consequently, the non-equilibrium effects are included in the calculation of e-ph coupling constant. The coupling model is verified by modeling the ultrafast dynamics in femtosecond pump-probe experiments on metal surface, which shows consistent results with the full integral treatment of scattering terms. The e-ph coupling constant is strongly reduced due to both the temporal non-equilibrium between different phonon branches and the spatial non-equilibrium of electrons in confined space. The present work will promote not only a fundamental understanding of the e-ph coupling constant but also the theoretical description of coupled electron and phonon transport at micro- and nanoscale.

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Wuli Miao, Moran Wang. 2020-12-30. Non-equilibrium effects on electron-phonon coupling constant in metals. https://doi.org/10.1103/physrevb.103.125412

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