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arXiv · 2101.01448

Four-Dimensional Imaging of Lattice Dynamics using Inelastic Scattering

Navdeep Rana·Aditya Prasad Roy·Dipanshu Bansal·Gopal Dixit
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Abstract

Time-resolved mapping of lattice dynamics in real- and momentum-space is essential to understand better several ubiquitous phenomena such as heat transport, displacive phase transition, thermal conductivity, and many more. In this regard, time-resolved diffraction and microscopy methods are employed to image the induced lattice dynamics within a pump-probe configuration. In this work, we demonstrate that inelastic scattering methods, with the aid of theoretical simulation, are competent to provide similar information as one could obtain from the time-resolved diffraction and imaging measurements. To illustrate the robustness of the proposed method, our simulated result of lattice dynamics in germanium is in excellent agreement with the time-resolved x-ray diffuse scattering measurement performed using x-ray free-electron laser. For a given inelastic scattering data in energy and momentum space, the proposed method is useful to image in-situ lattice dynamics under different environmental conditions of temperature, pressure, and magnetic field. Moreover, the technique will profoundly impact where time-resolved diffraction within the pump-probe setup is not feasible, for instance, in inelastic neutron scattering.

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Navdeep Rana, Aditya Prasad Roy, Dipanshu Bansal, Gopal Dixit. 2021-01-05. Four-Dimensional Imaging of Lattice Dynamics using Inelastic Scattering. https://doi.org/10.1038/s41524-020-00475-4

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