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arXiv · 2102.04612

Successive destruction of charge density wave states by pressure in LaAgSb$_2$

Kazuto Akiba·Hiroaki Nishimori·Nobuaki Umeshita·Tatsuo C. Kobayashi
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Abstract

We comprehensively studied the magnetotransport properties of LaAgSb$_2$ under high pressure up to 4 GPa, which showed unique successive charge density wave (CDW) transitions at $T_{CDW1}\sim 210$ K and $T_{CDW2}\sim 190$ K at ambient pressure. With the application of pressure, both $T_{CDW1}$ and $T_{CDW2}$ were suppressed and disappeared at the critical pressures of $P_{CDW1}=3.0$--3.4 GPa and $P_{CDW2}=1.5$--1.9 GPa, respectively. At $P_{CDW1}$, the Hall conductivity showed a step-like increase, which is consistently understood by the emergence of two-dimensional hollow Fermi surface at $P_{CDW1}$. We also observed a significant negative magnetoresistance effect when the magnetic field and current were applied parallel to the $c$ axis. Shubnikov--de Haas (SdH) oscillation measurements under pressure directly showed the changes in the Fermi surface across the CDW phase boundaries. In $P P_{CDW1}$, we observed a single frequency of $\sim 48$ T with a cyclotron effective mass of 0.066 $m_0$, whose cross section in the reciprocal space corresponded to only 0.22\% of the first Brillouin zone. Besides, we observed another oscillation component with frequency of $\sim 9.2$ T, which is significantly enhanced in the limited pressure range of $P_{CDW2}<P<P_{CDW1}$. The amplitude of this oscillation was anomalously suppressed in the high-field and low-temperature region, which cannot be explained by the conventional Lifshitz--Kosevich formula.

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Kazuto Akiba, Hiroaki Nishimori, Nobuaki Umeshita, Tatsuo C. Kobayashi. 2021-02-24. Successive destruction of charge density wave states by pressure in LaAgSb$_2$. https://doi.org/10.1103/physrevb.103.085134

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