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arXiv · 2102.12291

Quantum paramagnetism and magnetization plateaus in a kagome-honeycomb Heisenberg antiferromagnet

Meghadeepa Adhikary·Arnaud Ralko·Brijesh Kumar
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Abstract

A spin-1/2 Heisenberg model on honeycomb lattice is investigated by doing triplon analysis and quantum Monte Carlo calculations. This model, inspired by Cu$_2$(pymca)$_3$(ClO$_4$), has three different antiferromagnetic exchange interactions ($J_A$, $J_B$, $J_C$) on three different sets of nearest-neighbour bonds which form a kagome superlattice. While the model is bipartite and unfrustrated, its quantum phase diagram is found to be dominated by a quantum paramagnetic phase that is best described as a spin-gapped hexagonal-singlet state. The N\'eel antiferromagnetic order survives only in a small region around $J_A=J_B=J_C$. The magnetization produced by external magnetic field is found to exhibit plateaus at 1/3 and 2/3 of the saturation value, or at 1/3 alone, or no plateaus. Notably, the plateaus exist only inside a bounded region within the hexagonal-singlet phase. This study provides a clear understanding of the spin-gapped behaviour and magnetization plateaus observed in Cu$_2$(pymca)$_3$(ClO$_4$), and also predicts the possible disappearance of 2/3 plateau under pressure.

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Meghadeepa Adhikary, Arnaud Ralko, Brijesh Kumar. 2021-02-24. Quantum paramagnetism and magnetization plateaus in a kagome-honeycomb Heisenberg antiferromagnet. https://doi.org/10.1103/physrevb.104.094416

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