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arXiv · 2103.09702

Imaging non-radiative point defects buried in quantum wells using cathodoluminescence

Thomas Weatherley·Wei Liu·Vitaly Osokin·Duncan Alexander·Robert Taylor·Jean-François Carlin·Raphaël Butté·Nicolas Grandjean
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Abstract

Crystallographic point defects (PDs) can dramatically decrease the efficiency of optoelectronic semiconductor devices, many of which are based on quantum well (QW) heterostructures. However, spatially resolving individual non-radiative PDs buried in such QWs has so far not been demonstrated. Here, using high-resolution cathodoluminescence (CL) and a specific sample design, we spatially resolve, image, and analyse non-radiative PDs in InGaN/GaN QWs. We identify two different types of PD by their contrasting behaviour with temperature, and measure their densities from $10^{14}$ cm$^{-3}$ to as high as $10^{16}$ cm$^{-3}$. Our CL images clearly illustrate the interplay between PDs and carrier dynamics in the well: increasing PD concentration severely limits carrier diffusion lengths, while a higher carrier density suppresses the non-radiative behaviour of PDs. The results in this study are readily interpreted directly from CL images, and represent a significant advancement in nanoscale PD analysis.

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Thomas Weatherley, Wei Liu, Vitaly Osokin, Duncan Alexander, Robert Taylor, Jean-François Carlin, Raphaël Butté, Nicolas Grandjean. 2021-03-17. Imaging non-radiative point defects buried in quantum wells using cathodoluminescence. https://doi.org/10.1021/acs.nanolett.1c01295

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