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arXiv · 2104.03941

Evidence for magnetic clusters in stoichiometric quantum critical CeRu$_2$Si$_2$

Alex Bretaña·Sean Fayfar·Wouter Montfrooij
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Abstract

Systems that have been prepared to undergo a second-order phase transition at zero Kelvin, the so-called quantum critical systems, appear to fall into two categories: (chemically) heavily-doped systems where the unusual properties can be related to a disorder-induced distribution of Kondo shielding temperatures, and (almost) stoichiometric systems where the departures from Fermi-liquid theory have been attributed to intrinsic instabilities. Here we show that this distinction is not as clear cut and that magnetic clusters associated with a distribution of Kondo shielding temperatures are also present in CeRu$_2$Si$_2$, a system close to a quantum critical point. By revisiting published data on this system and comparing them to the results for heavily-doped quantum critical Ce(Ru$_{0.755}$Fe$_{0.245}$)$_2$Ge$_2$, we show that clusters exist in both systems at low temperatures, and that the moments of the Ce-ions within these clusters have all lined up with their neighbors. This implies that the dominant physics that drives heavily-doped systems, namely spontaneous formation of magnetic clusters, should also play a leading role in the response of homogenous systems. This represents a notable departure of how the physics that governs quantum critical points is treated in the literature.

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Alex Bretaña, Sean Fayfar, Wouter Montfrooij. 2021-04-08. Evidence for magnetic clusters in stoichiometric quantum critical CeRu$_2$Si$_2$. https://doi.org/10.1103/physrevb.104.085135

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