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arXiv · 2104.04573

Polarons formation in Bi-deficient BaBiO$_3$

W. Román Acevedo·S. Di Napoli·F. Romano·G. Rodríguez Ruiz·P. Nukala·C. Quinteros·J. Lecourt·U. Lüders·V. Vildosola·D. Rubi
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Abstract

BaBiO$_3$ is a charged ordered Peierls-like perovskite well known for its superconducting properties upon K or Pb doping. We present a study on the transport and electronic properties of BaBiO$_3$ perovskite with strong Bi-deficiency. We show that it is possible to synthesize BaBiO$_3$ thin layers with Bi-vacancies above 8-10% by depositing an yttrium-stabilized zirconia capping layer. By combining transport measurements with ab initio calculations we propose an scenario where the Bi-vacancies give rise to the formation of polarons and suggest that the electrical transport is dominated by the migration of these polarons trapped at Bi$^{3+}$ sites. Our work shows that cation vacancies engineering -- hardly explored to date -- appears as a promising pathway to tune the electronic and functional properties of perovskites.

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W. Román Acevedo, S. Di Napoli, F. Romano, G. Rodríguez Ruiz, P. Nukala, C. Quinteros, J. Lecourt, U. Lüders, V. Vildosola, D. Rubi. 2021-04-09. Polarons formation in Bi-deficient BaBiO$_3$. https://doi.org/10.1103/physrevb.104.125307

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