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arXiv · 2104.12812

A unified theory of spin and charge excitations in high-$T_c$ cuprates: Quantitative comparison with experiment and interpretation

M. Fidrysiak·J. Spałek
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Abstract

We provide a unified interpretation of both paramagnon and plasmon modes in high-$T_c$ copper-oxides, and verify it quantitatively against available resonant inelastic $x$-ray scattering (RIXS) data across the hole-doped phase diagram. Three-dimensional extended Hubbard model, with included long-range Coulomb interactions and doping-independent microscopic parameters for both classes of quantum fluctuations, is used. Collective modes are studied using VWF+$1/\mathcal{N}_f$ approach which extends variational wave function (VWF) scheme by means of an expansion in inverse number of fermionic flavors ($1/\mathcal{N}_f$). We show that intense paramagnons persist along the anti-nodal line from the underdoped to overdoped regime and undergo rapid overdamping in the nodal direction. Plasmons exhibit a three-dimensional character, with minimal energy corresponding to anti-phase oscillations on neighboring $\mathrm{CuO_2}$ planes. The theoretical spin- and charge excitation energies reproduce semi-quantitatively RIXS data for $\mathrm{(Bi, Pb)_2 (Sr, La)_2 CuO_{6+δ}}$. The present VWF+$1/\mathcal{N}_f$ analysis of dynamics and former VWF results for static quantities combine into a consistent description of the principal properties of hole-doped high-$T_c$ cuprates as strongly correlated systems.

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M. Fidrysiak, J. Spałek. 2021-04-26. A unified theory of spin and charge excitations in high-$T_c$ cuprates: Quantitative comparison with experiment and interpretation. https://doi.org/10.1103/physrevb.104.l020510

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