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arXiv · 2107.00419

Orbitally-selective Breakdown of the Fermi Liquid and Simultaneous Enhancement of Metallic and Insulating States in Correlated Multi-band Systems with Spin-orbit Coupling

Ze-Yi Song·Xiu-Cai Jiang·Yu-Zhong Zhang
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Abstract

We show that spin-orbit coupling (SOC) plays Janus-faced roles on the orbitally-selective Mott transitions in a three-orbital Hubbard model with crystal field splitting at a specific filling of $2/3$, which is a minimal Hamiltonian for ruthenates. While the SOC favors metallic state due to enhancement of orbital hybridization at smaller on-site Coulomb repulsions, it stabilizes the Mott insulating state ascribed to lifting of orbital degeneracies and enhancement of band polarizations at larger electronic interaction. Moreover, an orbitally-selective non-Fermi liquid (OSnFL), where breakdown and retention of the Fermi liquid coexist in different orbitals, emerges between the orbitally-selective Mott phase and the Fermi-liquid state. This novel state can be used to account for the exotic metallic behavior observed in 4$d$ materials, such as Ca$_{1.8}$Sr$_{0.2}$RuO$_4$, Ba$_2$RuO$_4$ under strain and Sr$_2$RuO$_4$ under uniaxial pressure. We propose that orbitally-selective Kondo breakdown may account for the OSnFL.

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Ze-Yi Song, Xiu-Cai Jiang, Yu-Zhong Zhang. 2021-07-01. Orbitally-selective Breakdown of the Fermi Liquid and Simultaneous Enhancement of Metallic and Insulating States in Correlated Multi-band Systems with Spin-orbit Coupling. https://doi.org/10.1103/physrevb.102.245124

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