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arXiv · 2107.04256

Interferometric mass spectrometry

Radu Ionicioiu
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Abstract

Accelerator mass spectrometry (AMS) is a widely-used technique with multiple applications, including geology, molecular biology and archeology. In order to achieve a high dynamic range, AMS requires tandem accelerators and large magnets, which thus confines it to big laboratories. Here we propose interferometric mass spectrometry (Interf-MS), a novel method of mass separation which uses quantum interference. Interf-MS employs the wave-like properties of the samples, and as such is complementary to AMS, in which samples are particle-like. This complementarity has two significant consequences: (i) in Interf-MS separation is performed according to the absolute mass $m$, and not to the mass-to-charge ratio $m/q$, as in AMS; (ii) in Interf-MS the samples are in the low-velocity regime, in contrast to the high-velocity regime used in AMS. Potential applications of Interf-MS are compact devices for mobile applications, sensitive molecules that break at the acceleration stage and neutral samples which are difficult to ionise.

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Radu Ionicioiu. 2021-07-09. Interferometric mass spectrometry. https://doi.org/10.1021/jasms.3c00105

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