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arXiv · 2108.11229

Stochastic Variational Approach to Small Atoms and Molecules Coupled to Quantum Field Modes

Alexander Ahrens·Chenhang Huang·Matt Beutel·Cody Covington·Kalman Varga
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Abstract

In this work, we present a stochastic variational calculation (SVM) of energies and wave functions of few particle systems coupled to quantum fields in cavity QED. The light-matter coupled system is described by the Pauli-Fierz Hamiltonian. The spatial wave function and the photon spaces are optimized by a random selection process. Examples for a two-dimensional trion and confined electrons as well as for the He atom and the Hydrogen molecule are presented showing that the light-matter coupling drastically changes the electronic states.

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Alexander Ahrens, Chenhang Huang, Matt Beutel, Cody Covington, Kalman Varga. 2021-08-25. Stochastic Variational Approach to Small Atoms and Molecules Coupled to Quantum Field Modes. https://doi.org/10.1103/physrevlett.127.273601

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