arXiv · 2206.00500
Spatial properties of entangled two-photon absorption
Abstract
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single- and two-photon absorption processes. We demonstrate that the entangled two-photon absorption shares a beam waist dependence similar to that of classical two-photon absorption. This result presents an additional argument for the wide range of contrasting values of quoted entangled two-photon absorption cross-sections of dyes in literature.
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D. Tabakaev, A. Djorovic, L. La Volpe, G. Gaulier, S. Ghosh, L. Bonacina, J. -P. Wolf, H. Zbinden, R. T. Thew. 2022-06-01. Spatial properties of entangled two-photon absorption. https://arxiv.org/abs/2206.00500
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