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arXiv · 2208.05702

Tunable electronic and magnetic phases in layered ruthenates: SrRuO3-SrTiO3 heterostructure upon strain

Minjae Kim·Chang-Jong Kang·Jae-Ho Han·Kyoo Kim·Bongjae Kim
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Abstract

Layered ruthenates are a unique class of systems which manifests a variety of electronic and magnetic features emerged from competing energy scales. At the heart of such features lies the multi-orbital physics, especially, the orbital-selective behavior. Here, we propose that the SrRuO3-SrTiO3 heterostructure is a highly tunable platform to obtain the various emergent properties. Employing the density functional theory plus dynamical mean-field theory, we thoroughly investigate the orbital-dependent physics of the system and identify the competing magnetic fluctuations. We show that the epitaxial strain drives the system towards multi-orbital or orbital selective Mott phases from the Hund metal regime. At the same time, the two different types of static magnetism are stabilized, ferromagnetism and checkerboard antiferromagnetism, from the competition with the spin-density wave instability.

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Minjae Kim, Chang-Jong Kang, Jae-Ho Han, Kyoo Kim, Bongjae Kim. 2022-08-11. Tunable electronic and magnetic phases in layered ruthenates: SrRuO3-SrTiO3 heterostructure upon strain. https://doi.org/10.1103/physrevb.106.l201103

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